Modeling and Mapping of Atmospheric Mercury Deposition in Adirondack Park, New York

Xue Yu, Charles T. Driscoll, Jiaoyan Huang, Thomas M. Holsen, Bradley D. Blackwell

Research output: Contribution to journalArticle

20 Scopus citations

Abstract

The Adirondacks of New York State, USA is a region that is sensitive to atmospheric mercury (Hg) deposition. In this study, we estimated atmospheric Hg deposition to the Adirondacks using a new scheme that combined numerical modeling and limited experimental data. The majority of the land cover in the Adirondacks is forested with 47% of the total area deciduous, 20% coniferous and 10% mixed. We used litterfall plus throughfall deposition as the total atmospheric Hg deposition to coniferous and deciduous forests during the leaf-on period, and wet Hg deposition plus modeled atmospheric dry Hg deposition as the total Hg deposition to the deciduous forest during the leaf-off period and for the non-forested areas year-around. To estimate atmospheric dry Hg deposition we used the Big Leaf model. The average atmospheric Hg deposition to the Adirondacks was estimated as 17.4 μg m-2 yr-1 with a range of -3.7-46.0 μg m-2 yr-1. Atmospheric Hg dry deposition (370 kg yr-1) was found to be more important than wet deposition (210 kg yr-1) to the entire Adirondacks (2.4 million ha). The spatial pattern showed a large variation in atmospheric Hg deposition with scattered areas in the eastern Adirondacks having total Hg deposition greater than 30 μg m-2 yr-1, while the southwestern and the northern areas received Hg deposition ranging from 25-30 μg m-2 yr-1.

Original languageEnglish (US)
Article numbere59322
JournalPloS one
Volume8
Issue number3
DOIs
StatePublished - Mar 25 2013

ASJC Scopus subject areas

  • Biochemistry, Genetics and Molecular Biology(all)
  • Agricultural and Biological Sciences(all)

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