INVESTIGATION OF EMISSION REDUCTION AND POWER GENERATION ON ELECTROCHEMICAL CATALYTIC MEMBRANES WITH THE ADDITION OF PEROVSKITE NANOCRYSTALS

Aliza M. Willsey, Kassidy Fields, Thomas S. Welles, Hanjie Lin, Weiwei Zheng, Jeongmin Ahn

Research output: Chapter in Book/Entry/PoemConference contribution

Abstract

With the depletion of fossil fuel resources, as well as increasing global temperatures, the interest in sustainable energy is on the rise. Currently, cars are a significant source of harmful emissions due to the use of internal combustion engines. Incomplete combustion byproducts are extremely harmful to the environment and the population, with links to acid rain, smog, and respiratory issues. While green energy solutions, such as electric vehicles, are being developed, the treatment of exhaust can also be an effective way to reduce the release of emissions into the atmosphere. It has been shown that a solid oxide fuel cell (SOFC) is able to break down emissions, even exceeding the capability of typical exhaust treatment methods. An investigation into the usage of an SOFC as an exhaust treatment material has found that the amplification of a signal generated across the cell has an even greater effect on emission reduction. Here, the addition of cesium lead bromide (CsPbBr3) nanocrystals to the fuel cell is being investigated. The SOFC is tested as an exhaust treatment solution and as a power generation device in comparison to a typical SOFC without added CsPbBr3 nanocrystals. CsPbBr3 is a perovskite semiconductor, so it is expected to have an effect on the reactivity of the fuel cell. Investigating the effects of adding nanocrystals into a SOFC will lead to advancements in exhaust treatment systems as well as power generation systems. The work here will show a direct relationship between the quantity of nanocrystals contained in the SOFC to the emission reduction and power generation abilities of the SOFC.

Original languageEnglish (US)
Title of host publicationEnergy
PublisherAmerican Society of Mechanical Engineers (ASME)
ISBN (Electronic)9780791886687
DOIs
StatePublished - 2022
EventASME 2022 International Mechanical Engineering Congress and Exposition, IMECE 2022 - Columbus, United States
Duration: Oct 30 2022Nov 3 2022

Publication series

NameASME International Mechanical Engineering Congress and Exposition, Proceedings (IMECE)
Volume6

Conference

ConferenceASME 2022 International Mechanical Engineering Congress and Exposition, IMECE 2022
Country/TerritoryUnited States
CityColumbus
Period10/30/2211/3/22

Keywords

  • Nitric oxide emissions
  • electrochemistry
  • fuel lean exhaust treatment
  • perovskite-based materials
  • platinum group metal catalytic converters
  • power generation
  • semiconductors
  • three-way catalytic converter

ASJC Scopus subject areas

  • Mechanical Engineering

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